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Dynamic x-ray diffraction computed tomography reveals real-time insight into catalyst active phase evolution

Jacques, S.D.M. and di Michiel, M. and Beale, A.M. and Sochi, Taha and O’Brien, M.G. and Espinosa Alonso, L. and Weckhuysen, B.M. and Barnes, Paul (2011) Dynamic x-ray diffraction computed tomography reveals real-time insight into catalyst active phase evolution. Angewandte Chemie - International Edition 50 (43), pp. 10148-10152. ISSN 1433-7851.

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Official URL: http://dx.doi.org/10.1002/anie.201106511

Abstract

Color X-ray images can be obtained by X-ray diffraction computed tomography (XRD-CT) where the mapping of the diffraction signal from the interiors of solid objects enables material-specific imaging. In their Communication on page 10 148 ff., S. D. M. Jacques et al. describe the first time-resolved XRD-CT experiment, which reveals the mechanism by which a catalyst evolves from its precursor during the preparation of millimeter-sized industrial hydrogenation catalyst body.

Item Type: Article
Keyword(s) / Subject(s): catalyst preparation, chemical imaging, computed tomography, heterogeneous catalysis, X-ray diffraction
School or Research Centre: Birkbeck Schools and Research Centres > School of Science > Biological Sciences
Depositing User: Administrator
Date Deposited: 15 Nov 2011 10:31
Last Modified: 17 Apr 2013 12:21
URI: http://eprints.bbk.ac.uk/id/eprint/4317

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